- Sabotage Plan (1938–40) 1
- Said, Hussein Ghassan 1, 2
- Salter, William 1
- Sánchez, Ilich Ramírez (Carlos the Jackal) 1
- SAS 1, 2
- Scargill, Arthur 1
- Schroeder, Frederick Adolphus 1
- Schultz, Max 1
- Scott, Harold 1
- Scott, Russell 1, 2
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- Secret Agent, The (Joseph Conrad) 1, 2
- Secret Intelligence Service 1, 2, 3, 4
- secret registry 1
- Secret Service Bureau 1
- Secret Service Committee (1919) 1
- Secret Service Committee (1921) 1
- Secret Service Committee (1925) 1
- Shaw, George Bernard 1
- Shelepin, Alexander 1
- Shepherd, William 1, 2
- Sherry, Peter 1
- Sidney Street siege (1911) 1
- Simpson, Colin 1
- Sinclair, Hugh 1, 2
- Sinn Féin 1, 2, 3, 4, 5, 6
- Skardon, Jim 1, 2, 3
- Smith, ‘Fergie’ 1, 2
- Smith, G. G. (Moonraker) 1, 2, 3
- Smith, Michael John 1
- Smither, Peter 1
- Special Branch Registry 1
- Special Demonstration Squad 1, 2
- Special Escort Group 1
- Special Irish Branch (SIB) 1, 2, 3, 4, 5, 6, 7, 8, 9
- renamed Special Branch 1
- Special Patrol Group (SPG) 1
- Spooner, Reg 1, 2
- SS1/SS2 1, 2, 3
- Stalin, Joseph 1
- state occasions 1
- Steinhauer, Gustav 1
- Stern Gang 1
- STILL LIFE operations 1
- ‘Stop the Seventy Tour’ campaign 1
- Suffragette movement 1, 2
- Sullivan, Pat 1
- Sullom Voe bomb plot (1981) 1
- surveillance 1
- Sweeney, John 1, 2, 3, 4, 5, 6, 7, 8, 9, 10, 11